• Core Journal of China
  • DOAJ
  • Scopus
  • Chinese Scientific and Technical Papers and Citations (CSTPC)
  • Chinese Science Citation Database (CSCD)
Advanced Search
XUE Yuan, YANG Yong-liang, WAN Kui-yuan, WU Xue-li, ZHU Xiao-hua, WANG Xiao-chun, LUO Song-guang. Preliminary Study on Distribution of Organochlorine Pesticides and Polychlorinated Biphenyls in Surface Soils and Atmosphere Along the Xihe River in Shenyang City[J]. Rock and Mineral Analysis, 2011, 30(1): 27-32.
Citation: XUE Yuan, YANG Yong-liang, WAN Kui-yuan, WU Xue-li, ZHU Xiao-hua, WANG Xiao-chun, LUO Song-guang. Preliminary Study on Distribution of Organochlorine Pesticides and Polychlorinated Biphenyls in Surface Soils and Atmosphere Along the Xihe River in Shenyang City[J]. Rock and Mineral Analysis, 2011, 30(1): 27-32.
shu

Preliminary Study on Distribution of Organochlorine Pesticides and Polychlorinated Biphenyls in Surface Soils and Atmosphere Along the Xihe River in Shenyang City

  • 1.

    College of Chemical and Environmental and Engineering, Qingdao University, Qingdao 266071, China

  • 2.

    Key Laboratory of Eco-Geochemistry, Chinese Academy of Geological Sciences, National Research Center for Geoanalysis, Beijing 100037, China

  • 3.

    Key Laboratory of Eco-Geochemistry, Chinese Academy of Geological Sciences, National Research Center for Geoanalysis, Beijing 100037, China

  • 4.

    College of Chemical and Environmental and Engineering, Qingdao University, Qingdao 266071, China

  • 5.

    Key Laboratory of Eco-Geochemistry, Chinese Academy of Geological Sciences, National Research Center for Geoanalysis, Beijing 100037, China

  • 6.

    Key Laboratory of Eco-Geochemistry, Chinese Academy of Geological Sciences, National Research Center for Geoanalysis, Beijing 100037, China

  • 7.

    Key Laboratory of Eco-Geochemistry, Chinese Academy of Geological Sciences, National Research Center for Geoanalysis, Beijing 100037, China

  • 8.

    Key Laboratory of Eco-Geochemistry, Chinese Academy of Geological Sciences, National Research Center for Geoanalysis, Beijing 100037, China

  • 9.

    Key Laboratory of Eco-Geochemistry, Chinese Academy of Geological Sciences, National Research Center for Geoanalysis, Beijing 100037, China

More Information
  • Received Date: August 15, 2010
  • Revised Date: October 28, 2010
    Abstract
  • The concentration of organochlorine pesticides (OCPs) and polychlorinated biphenyls (PCBs) in surface soils and atmosphere along the Xihe River in Shenyang city were determined to study the residual levels and environmental behaviors of these compounds. Concentrations of HCHs and DDTs were in the range of 2.32~15.90 ng/g with average value of 8.99 ng/g and 9.06~111.6 ng/g with average value of 37.08 ng/g, respectively. The mean concentration of 7 kinds of PCBs was 1.01 ng/g. Results showed that concentrations of OCPs and PCBs in most sampling sites did not exceed the limits of the national environment quality standards for soils. The results also indicated that although lindane might be used in recent years no DDTs input from new pollution sources were found. And DDTs residuals in soils from some sites posed a potential threatening to the ecosystem. The mean concentrations of HCHs, DDTs and PCBs in air samples were 18.97 ng/m3, 42.27 ng/m3 and 20.59 ng/m3 respectively, which means that long distance atmospheric transport of the OCPs may play a significant role in pollution in these areas. The fugacity model was used to study the environmental behaviors of HCHs and DDTs and escaping tendency of HCHs and DDTs from soils to ambient air was found in the studied area.
    • FullText(HTML)
    • References (31)
  • 宋雪英,孙丽娜,王鑫,李昕馨,孙铁珩.细河河水及其沿岸地下水水质的有机污染特征[J].生态学杂志,2007,26(12):2057-2061.
    刘韬,郭淑满.污水灌溉对沈阳市农田土壤中重金属含量的影响[J].环境保护科学,2003,29(6):51-52.
    杨继松,孙丽娜,杨晓波,马力.沈阳市细河沿岸农田土壤重金属污染评价[J].农业环境科学学报,2007,26(5):1933-1936.
    路国慧,杨永亮,刘晓端,黄毅,何俊,徐清,黄园英.沈阳地区河水及沿岸地下水中卤代烃的污染特征[J].岩矿测试,2009,28(4):316-320.
    杨永亮,路国慧,杨伟贤,潘静,谷保佐知,山下信义,林群声.沈阳地区水环境和生物样品中全氟化合物的污染分布特征[J].环境科学学报,2010,30(9):1-11.
    刘韬,郭淑满.污水灌溉对沈阳市农田土壤中重金属含量的影响[J].环境保护科学,2003,29(6):51-52.
    杨继松,孙丽娜,杨晓波,马力.沈阳市细河沿岸农田土壤重金属污染评价[J].农业环境科学学报,2007,26(5):1933- 1936.
    仲夏,索丽珍,于凤玲.沈阳市农田土壤农药残留水平[J].农村生态环境,1996,12(4): 58-60.
    Wania F, Shen L, Lei Y D, Camilla T, Muir D C G. Development and calibration of a resin-based passive sampling system for monitoring persistent organic pollutants in the atmosphere[J].Environmental Science and Technology, 2003, 37: 1352-1359.

    Wania F, Shen L, Lei Y D, Camilla T, Muir D C G. Development and calibration of a resin-based passive sampling system for monitoring persistent organic pollutants in the atmosphere[J].Environmental Science and Technology, 2003, 37: 1352-1359.
    耿存珍,李明伦,杨永亮,张利锋,聂丽曼.青岛地区土壤中OCPs和PCBs污染现状研究[J].青岛大学学报:工程技术版,2006,21(2):42-48.
    朱晓华,杨永亮,路国慧,吴学丽,何俊,罗松光.广州市海珠区有机氯农药污染状况及其土-气交换[J].岩矿测试,2010,28(2):91-96.
    WHO. Environmental health criteria 83 (DDT and its deriva-tives-environmental aspects) .Geneva,1989:14-151.

    WHO. Environmental health criteria 83 (DDT and its deriva-tives-environmental aspects) .Geneva,1989:14-151.
    章海波,骆永明,滕应,赵其国,万洪富.珠江三角洲地区典型类型土壤中DDT残留及其潜在风险[J].土壤,2006,38(5): 547-551.
    邱黎敏,张建英,骆永明.浙北农田土壤中HCH和DDT的残留及其风险[J].农业环境科学学报,2005,24(6):1161-1165.
    Shen L, Wania F.Compilation, evaluation, and selection of physical-chemical property data for organochlorine pesticides[J].Journal of Chemical and Engineering Data, 2005, 50:742-768

    Shen L, Wania F.Compilation, evaluation, and selection of physical-chemical property data for organochlorine pesticides[J].Journal of Chemical and Engineering Data, 2005, 50:742-768
    Middeldorp P J M, Jaspers M, Zehnder A J B, Schraa G. Biotransformation of α-, β-, γ-, and δ-hexachlorocyclohexane under methanogenic conditions[J]. Environmental Science and Technology, 1996, 30:2345-2349.

    Middeldorp P J M, Jaspers M, Zehnder A J B, Schraa G. Biotransformation of α-, β-, γ-, and δ-hexachlorocyclohexane under methanogenic conditions[J]. Environmental Science and Technology, 1996, 30:2345-2349.
    Kalbitz K, Popp P, Geyer W, Hanschmann G.β-HCH mobilization in polluted wetland soils as influenced by dissolved organic matter[J].Science of the Total Environment, 1997, 204: 37-48.

    Kalbitz K, Popp P, Geyer W, Hanschmann G.β-HCH mobilization in polluted wetland soils as influenced by dissolved organic matter[J].Science of the Total Environment, 1997, 204: 37-48.
    Hong H, Xu L, Zhang L, Chen J C, Wong Y S, Wan T S M. Environmental fate and chemistry of organic pollutants in the sediment of Xiamen and Victoria Harbors[J]. Marine Pollution Bulletin, 1995, 31: 229-236.

    Hong H, Xu L, Zhang L, Chen J C, Wong Y S, Wan T S M. Environmental fate and chemistry of organic pollutants in the sediment of Xiamen and Victoria Harbors[J]. Marine Pollution Bulletin, 1995, 31: 229-236.
    Qiu X H, Zhu T, Li J, Pan H S, Li Q L, Miao G F, Gong J C. Organochlorine pesticides in the air around the Taihu Lake, China[J].Environmental Science and Technology 2004, 38: 1368-1374.

    Qiu X H, Zhu T, Li J, Pan H S, Li Q L, Miao G F, Gong J C. Organochlorine pesticides in the air around the Taihu Lake, China[J].Environmental Science and Technology 2004, 38: 1368-1374.
    Urzelai A,Vega M, Angulo E. Deriving ecological risk-based soil quality values in the Basque county[J]. Science of the Total Environment, 2000,247(2): 279-284.

    Urzelai A,Vega M, Angulo E. Deriving ecological risk-based soil quality values in the Basque county[J]. Science of the Total Environment, 2000,247(2): 279-284.
    Jongbloed R H, Traas T P, Luttik R. A probabilistic model for deriving soil quality criteria based on secondary poisoning of top predators Ⅱ. Calculations for dichloro-dipheny- chloroethane (DDT) and cadmium[J].Ecotoxicology and Environment Safety, 1996, 34: 279-306.

    Jongbloed R H, Traas T P, Luttik R. A probabilistic model for deriving soil quality criteria based on secondary poisoning of top predators Ⅱ. Calculations for dichloro-dipheny- chloroethane (DDT) and cadmium[J].Ecotoxicology and Environment Safety, 1996, 34: 279-306.
    武振艳.吉林省典型地区土壤与农作物中有机氯农药和多氯联苯的分布特征 .长春:吉林农业大学,2010:1-85.
    Li J, Zhang G, Guo L L, Xu W H, Li X D, Lee C S L, Ding A J, Wang T. Organochlorine pesticides in the atmosphere of Guangzhou and Hong Kong: Regional sources and long-range atmospheric transport[J].Atmospheric Environment, 2007, 41:3889-3903.

    Li J, Zhang G, Guo L L, Xu W H, Li X D, Lee C S L, Ding A J, Wang T. Organochlorine pesticides in the atmosphere of Guangzhou and Hong Kong: Regional sources and long-range atmospheric transport[J].Atmospheric Environment, 2007, 41:3889-3903.
    李春雷,麦碧娴,郝永梅,盛国英,傅家谟.珠江三角洲空气中多氯联苯污染的区域背景研究[J].中国环境科学,2004,24(4):501-504.
    王俊,张干,李向东,李军,徐维海,郭玲利,余莉莉,钟流举,向运荣,彭永焯. 利用PUF被动采样技术监测珠江三角洲地区大气中多氯联苯分布[J].环境科学,2007,28(3): 973-976.
    Mackay D. Multimedia environmental models: The fugacity approach[M]. 2 ed. Lewis Publishers,2001.

    Mackay D. Multimedia environmental models: The fugacity approach[M]. 2 ed. Lewis Publishers,2001.
    Mackay D. Finding fugacity feasible[J].Environmental Science and Technology, 1979, 13: 1218-1223.

    Mackay D. Finding fugacity feasible[J].Environmental Science and Technology, 1979, 13: 1218-1223.
    Wang X L, Tao S, Xu F L, Dawson R W, Cao J, Li B G, Fang Y. Modeling the fate of benzo - pyrene in the wastewater-irrigated areas of Tianjin with a fugacity model[J].Journal of Environmental Quality,2002,31:896-903.

    Wang X L, Tao S, Xu F L, Dawson R W, Cao J, Li B G, Fang Y. Modeling the fate of benzo - pyrene in the wastewater-irrigated areas of Tianjin with a fugacity model[J].Journal of Environmental Quality,2002,31:896-903.
    曹红英,龚钟明,曹军,李本纲,徐福留,陶澍.估算天津环境中γ-HCH归宿的逸度模型[J].环境科学,2003,24(2): 77-81.
    Bruhn R, Lakaschus S, McLachlan M S. Air/sea gas exchange of PCBs in the southern Baltic Sea[J].Atmospheric Environment,2003,37:3445-3454.

    Bruhn R, Lakaschus S, McLachlan M S. Air/sea gas exchange of PCBs in the southern Baltic Sea[J].Atmospheric Environment,2003,37:3445-3454.
    Mackay D. Multimedia environmental models[M]. 2 ed. Lewis: Boca Raton,2001.

    Mackay D. Multimedia environmental models[M]. 2 ed. Lewis: Boca Raton,2001.
    • Related Articles

  • Related Articles

    [1]Zhen-kun WANG, Hong JIN, Xue-jun LI, Chi ZHANG, Xin SUN, Tao BIAN, Yu-qing MO, Qiang LUO. Study on Migration of Lead and Admium in the Port Environment and Model building[J]. Rock and Mineral Analysis, 2013, 32(5): 753-758.
    [2]SONG Xue-ying, JIN Cai-xia, HU Xiao-jun, LI Yu-shuang, LI Hui-ying, YANG Ji-song. Fuzzy Evaluation on the Water Quality of the Taizi River[J]. Rock and Mineral Analysis, 2011, 30(6): 705-708.
    [3]TONG Ling, WU Shu-qi, YANG Jia-jia, ZHANG Ling-jin. Determination of 25 Organochlorine Pesticides and Polychlorinated Biphenyls in Soils by Gas Chromatography[J]. Rock and Mineral Analysis, 2010, 29(3): 277-281.
    [4]WU Zhen-yan, YANG Yong-liang, AN Li-hua, JIAO Xing-chun, LU Guo-hui, LIU Xiao-duan, XU Qing, XIE Wen-ming. Distribution Characteristics of Organochlorine Pesticides and Polychlorinated Biphenyls in Top Soils from Development Zone in New Jiangwan City[J]. Rock and Mineral Analysis, 2010, 29(3): 231-235.
    [5]WANG Xiaochun, LU Guohui, LIU Xiaoduan, HE Jun, TANG Qifeng, XU Qing, LIU Jiuchen, LUO Songguang, YANG Yongliang. Vertical Distribution Characteristics and Speciation Analysis of Heavy Metals in Topsoils around Xihe River of Shenyang[J]. Rock and Mineral Analysis, 2010, 29(2): 97-103.
    [6]CHEN Bo, FENG Yongming, LIU Hongqing. Determination of Multi-elements in Airborne Dust with Air Filtrer Membrance Sampling[J]. Rock and Mineral Analysis, 2009, 28(5): 435-438.
    [7]Statistic Analysis of the Release Characteristics of Formaldehyde and Benzene in Indoor Air[J]. Rock and Mineral Analysis, 2008, 27(2): 158-160.
    [8]Determination of Vanadium in Geological Samples by Air Mixed Oxygen-Acetylene Flame Atomic Absorption Spectrometry[J]. Rock and Mineral Analysis, 2003, (4): 300-302.
    [9]Determination of Trace Barium in Geological Samples by Oxygen-Air-Acetylene Flame Atomic Absorption Spectrometry[J]. Rock and Mineral Analysis, 2002, (3): 187-189.
    [10]Effect of Air Bubbles on the Peak Shapes and Elimination of the Interferences in Flow Injection Analysis[J]. Rock and Mineral Analysis, 1996, (2): 104-108.
    • Supplements (0)

Catalog

    Get Citation
    PDF
    XML
    Article views (1927) PDF downloads (919) Cited by()
    Turn off MathJax
    Article Contents
    ABSTRACT
    References
    Related Articles

    Competent Authorities：China Association for Science and Technology

    Sponsored by：Geological Society of China; National Research Center for Geoanalysis

    Address：No. 26 Baiwanzhuang Road, Xicheng District, Beijing 100037, China Email：ykcs_zazhi@163.com Tel：010-68999562

    京公网安备 11010202008159号 京ICP备2022024991号

    Supported by: Beijing Renhe Information Technology Co., Ltd.  Baidu Analytics

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return