激光剥蚀-等离子体质谱技术及其在地球化学宇宙化学和环境研究中的应用

JOCHUM Klaus Peter; STOLL Brigitte; FRIEDRICH Jon M; AMINI Marghaleray; BECKER Stefan; DüCKING Marc; EBEL Denton S; ENZWEILER Jacinta; 胡明月; KUZMIN Dmitry; MERTZKRAUS Regina; MüLLER Werner E G; REGNERY Julia; SOBOLEV Alexander; 王晓红; 詹秀春

激光剥蚀-等离子体质谱技术及其在地球化学宇宙化学和环境研究中的应用

1.
Max-Planck-Institut für Chemie
2.
Max PlanckInstitut für Chemie
3.
Department of Earth and Planetary Sciences, American Museum of Natural History， Department of Chemistry, Fordham University
4.
Max-Planck-Institut für Chemie， Saskatchewan Isotope Laboratory, Department of Geological Sciences, University of 〖DW〗Saskatchewan
5.
Bundeskriminalamt
6.
Bundeskriminalamt
7.
Department of Earth and Planetary Sciences, American Museum of Natural History
8.
Instituto de Geociências, University of Campinas
9.
国家地质实验测试中心
10.
Max-Planck-Institut für Chemie，Institute of Geology and Mineralogy, Siberian Branch of Russian Academy of Sciences
11.
Institut für Geowissenschaften, Universit?t Mainz
12.
Institut für Physiologische Chemie, Universit?t Mainz
13.
Max-Planck-Institut für Chemie
14.
V.I. Vernadsky Institute of Geochemistry and Analytical Chemistry, Russian Academy of Sciences，Max-Planck-Institut für Chemie
15.
国家地质实验测试中心
16.
国家地质实验测试中心

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出版历程
- 收稿日期: 2008-09-26
- 修回日期: 2008-10-25

Laser Ablation-Inductively Coupled Plasma-Mass Spectrometry and Its Application in Geochemistry, Cosmochemistry and Environmental Research

1.
Max-Planck-Institut für Chemie
2.
Max PlanckInstitut für Chemie
3.
Department of Earth and Planetary Sciences, American Museum of Natural History， Department of Chemistry, Fordham University
4.
Max-Planck-Institut für Chemie， Saskatchewan Isotope Laboratory, Department of Geological Sciences, University of Saskatchewan
5.
Bundeskriminalamt
6.
Bundeskriminalamt
7.
Department of Earth and Planetary Sciences, American Museum of Natural History
8.
Instituto de Geociências, University of Campinas
9.
National Research Center for Geoanalysis
10.
Max-Planck-Institut für Chemie，Institute of Geology and Mineralogy, Siberian Branch of Russian Academy of Sciences
11.
Institut für Geowissenschaften, Universit?t Mainz
12.
Institut für Physiologische Chemie, Universit?t Mainz
13.
Max-Planck-Institut für Chemie
14.
V.I. Vernadsky Institute of Geochemistry and Analytical Chemistry, Russian Academy of Sciences，Max-Planck-Institut für Chemie
15.
National Research Center for Geoanalysis
16.
National Research Center for Geoanalysis

摘要

摘要: 激光剥蚀-等离子体质谱（LA-ICPMS）已成为地球化学、宇宙化学和环境研究领域元素和同位素原位分析最重要的技术之一。文章介绍了多种类型的质谱仪及其使用的激光器。用途最广的LA-ICPMS仪器之一是单接收器扇形磁场质谱仪，配有Nd:YAG激光剥蚀系统（激光波长分为193 nm和213 nm两种），MPI Mainz实验室使用的就是这套系统，文章对此作一详细介绍。文中阐述了数据优化技术及其多种校正过程；介绍LA-ICPMS在痕量元素和同位素分析领域的一些应用，包括参考物质的研制，Hawaiian玄武岩、Martian陨石、生物骨针和珊瑚虫中痕量元素分析及熔融包裹体和富钙-铝碳质球粒陨石中的铅和锶同位素测量。
- 激光剥蚀-等离子体质谱；地质样品；参考物质；陨石；生物样品；痕量元素； /
- 同位素比值
Abstract: Laser ablation (LA)-inductively coupled plasmamass spectrometry (ICP-MS) has become one of the most important methods for in situ trace elemental and isotopic analysis in geochemistry, cosmochemistry and environmental research. For these purposes, different kinds of mass spectrometers and lasers are used, which are presented in this paper. One of the most useful LA-ICPMS instruments is the combination of a single-collector sector field mass spectrometer with Nd:YAG laser ablation systems (193 nm and 213 nm wavelengths, respectively). This design used in the MPI Mainz laboratory is described in detail in this paper. Data optimization techniques including diverse correction procedures are also discussed. To demonstrate the power of LA-ICPMS, several applications of trace elemental and isotopic analysis are presented, such as investigations of reference materials, trace element analysis in Hawaiian basalts, Martian meteorites, biological spicules and corals, as well as Pb and Sr isotope measurements of melt inclusions and Ca-Al rich inclusions of carbonaceous chondrites.
- laser /
- ablation-inductively

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激光剥蚀-等离子体质谱技术及其在地球化学宇宙化学和环境研究中的应用

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Laser Ablation-Inductively Coupled Plasma-Mass Spectrometry and Its Application in Geochemistry, Cosmochemistry and Environmental Research

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